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    Experimental Study of the Incoherent Spectral Weight in the Photoemission Spectra of the Misfit Cobaltate [Bi2Ba2O4][CoO2]2

    A. Nicolaou1,2, V. Brouet1, M. Zacchigna3, I. Vobornik3, A. Tejeda2,4, A. Taleb-Ibrahimi2, P. Le Fèvre2, F. Bertran2, S. Hébert5 et al.

    H. Muguerra5 and D. Grebille5

    • 1Laboratoire de Physique des Solides, Université Paris-Sud, UMR8502, Bât 510, 91405 Orsay, France
    • 2Synchrotron SOLEIL, L’Orme des Merisiers, Saint-Aubin-BP48, 91192 Gif-sur-Yvette, France
    • 3CNR-INFM, Laboratorio Nazionale TASC c/o Area Science Park, strada statale 14 Kilometer 163.5, I-34012 Basovizza (TS), Italy
    • 4Institut Jean Lamour, CNRS-Nancy-Université-UPV-Metz, 54506 Vandoeuvre-les-Nancy, France
    • 5Laboratoire CRISMAT, UMR 6508 CNRS et Ensicaen, 14050 Caen, France

    Phys. Rev. Lett. 104, 056403 – Published 5 February, 2010

    DOI: https://doi.org/10.1103/PhysRevLett.104.056403

    Abstract

    Previous angle-resolved photoemission spectroscopy experiments in NaxCoO2 reported both a strongly renormalized bandwidth near the Fermi level and moderately renormalized Fermi velocities, leaving it unclear whether the correlations are weak or strong and how they could be quantified. We explain why this situation occurs and solve the problem by extracting clearly the coherent and incoherent parts of the band crossing the Fermi level. We show that one can use their relative weight to estimate self-consistently a quasiparticle weight Z=0.15±0.05. We suggest this method could be a reliable way to study the evolution of correlations in cobaltates and for comparison with other strongly correlated systems.

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